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We present results from two-photon photoassociative spectroscopy of the least-bound vibrational level of the X$^1Sigma_g^+$ state of the $^{88}$Sr$_2$ dimer. Measurement of the binding energy allows us to determine the s-wave scattering length, $a_{88}=-1.4(6) a_0$. For the intermediate state, we use a bound level on the metastable $^1S_0$-$^3P_1$ potential, which provides large Franck-Condon transition factors and narrow one-photon photoassociative lines that are advantageous for observing quantum-optical effects such as Autler-Townes resonance splittings.
We demonstrate photoassociation (PA) of ultracold fermionic $^{87}$Sr atoms. The binding energies of a series of molecular states on the $^1Sigma^+_u$ $5s^2,^1$S$_0+5s5p,^1$P$_1$ molecular potential are fit with the semiclassical LeRoy-Bernstein mode
We have produced large samples of ultracold $^{88}$Sr$_2$ molecules in the electronic ground state in an optical lattice. The molecules are bound by 0.05 cm$^{-1}$ and are stable for several milliseconds. The fast, all-optical method of molecule crea
We present two-photon photoassociation to the least-bound vibrational level of the X$^1Sigma_g^+$ electronic ground state of the $^{86}$Sr$_2$ dimer and measure a binding energy of $E_b=-83.00(7)(20)$,kHz. Because of the very small binding energy, th
We employ two-photon spectroscopy to study the vibrational states of the triplet ground state potential ($a^3Sigma^+$) of the $^{23}$Na$^{6}$Li molecule. Pairs of Na and Li atoms in an ultracold mixture are photoassociated into an excited triplet mol
We investigate the prospects of using two-mode intensity squeezed twin-beams, generated in Rb vapor, to improve the sensitivity of spectroscopic measurements by engaging two-photon Raman transitions. As a proof of principle demonstration, we demonstr