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تسجيل مستخدم جديد$^{77}$Se NMR investigation of the field-induced spin-density-wave transitions in (TMTSF)$_2$ClO$_4$
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Complementary $^{77}$Se nuclear magnetic resonance (NMR) and electrical transport have been used to correlate the spin density dynamics with the subphases of the field-induced spin density wave (FISDW) ground state in tmt. We find that the peaks in the spin-lattice relaxation rate 1/T$_1$ appear within the metal-FISDW phase boundary and/or at first-order subphase transitions. In the quantum limit above 25 T, the NMR data gives an insight into the FISDW electronic structure.
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We have investigated the origin of the large increase in spin-echo decay rates for the $^{77}$Se nuclear spins at temperatures near to $T=30K$ in the organic superconductor (TMTSF)$_2$ClO$_4$. The measured angular dependence of $T_2^{-1}$ demonstrate
s that the source of the spin-echo decays lies with carrier density fluctuations rather than fluctuations in TMTSF molecular orientation. The very long time scales are directly associated with the dynamics of the anion ordering occurring at $T=25K$, and the inhomogeneously broadened spectra at lower temperatures result from finite domain sizes. Our results are similar to observations of line-broadening effects associated with charge-ordering transitions in quasi-two dimensional organic conductors.
We have performed $^{77}$Se NMR on a single crystal sample of the field induced superconductor $lambda$-(BETS)$_{2}$FeCl$_{4}$. Our results obtained in the paramagnetic state provide a microscopic insight on the exchange interaction $J$ between the s
pins textbf{s} of the BETS $pi$ conduction electrons and the Fe localized $d$ spins textbf{S}. The absolute value of the Knight shift textbf{K} decreases when the polarization of the Fe spins increases. This reflects the ``negative spin polarization of the $pi$ electrons through the exchange interaction $J$. The value of $J$ has been estimated from the temperature and the magnetic field dependence of textbf{K} and found in good agreement with that deduced from transport measurements (L. Balicas textit{et al}. Phys. Rev. Lett. textbf{87}, 067002 (2001)). This provides a direct microscopic evidence that the field induced superconductivity is due to the compensation effect predicted by Jaccarino and Peter (Phys. Rev. Lett. textbf{9}, 290 (1962)). Furthermore, an anomalous broadening of the NMR line has been observed at low temperature, which suggests the existence of charge disproportionation in the metallic state neighboring the superconducting phase.
Magnetoresistance measurements have been carried out along the highly conducting a axis in the FISDW phase of hydrogened and deuterated (TMTSF)$_2$ClO$_4$ for various cooling rates through the anion ordering temperature. With increasing the cooling r
ate, a) the high field phase boundary $beta_{rm {HI}}$, observed at 27 T in hydrogened samples for slowly cooled, is shifted towards a lower field, b) the last semimetallic SDW phase below $beta_{rm {HI}}$ is suppressed, and c) the FISDW insulating phase above $beta_{rm {HI}}$ is enhanced in both salts. The cooling rate dependence of the FISDW transition and of $beta_{rm {HI}}$ in both salts can be explained by taking into account the peculiar SDW nesting vector stabilized by the dimerized gap due to anion ordering.
Magnetoresistance measurements on the quasi one-dimensional organic conductor (TMTSF)_2PF_6 performed in magnetic fields B up to 16T, temperatures T down to 0.12K and under pressures P up to 14kbar have revealed new phases on its P-B-T phase diagram.
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