Self-referencing a continuous-wave laser with electro-optic modulation

We phase-coherently measure the frequency of continuous-wave (CW) laser light by use of optical-phase modulation and f-2f nonlinear interferometry. Periodic electro-optic modulation (EOM) transforms the CW laser into a continuous train of picosecond optical pulses. Subsequent nonlinear-fiber broadening of this EOM frequency comb produces a supercontinuum with 160 THz of bandwidth. A critical intermediate step is optical filtering of the EOM comb to reduce electronic-noise-induced decoherence of the supercontinuum. Applying f-2f self-referencing with the supercontinuum yields the carrier-envelope offset frequency of the EOM comb, which is precisely the difference of the CW laser frequency and an exact integer multiple of the EOM pulse repetition rate. Here we demonstrate absolute optical frequency metrology and synthesis applications of the self-referenced CW laser with <5E-14 fractional accuracy and stability.

Phase Steps and Hot Resonator Detuning in Microresonator Frequency Combs

Experiments and theoretical modeling yielded significant progress towards understanding of Kerr-effect induced optical frequency comb generation in microresonators. However, the simultaneous interaction of hundreds or thousands of optical comb frequencies with the same number of resonator modes leads to complicated nonlinear dynamics that are far from fully understood. An important prerequisite for modeling the comb formation process is the knowledge of phase and amplitude of the comb modes as well as the detuning from their respective microresonator modes. Here, we present comprehensive measurements that fully characterize optical microcomb states. We introduce a way of measuring resonator dispersion and detuning of comb modes in a hot resonator while generating an optical frequency comb. The presented phase measurements show unpredicted comb states with discrete {pi} and {pi}/2 steps in the comb phases that are not observed in conventional optical frequency combs.

A microresonator frequency comb optical clock

Optical-frequency combs enable measurement precision at the 20th digit, and accuracy entirely commensurate with their reference oscillator. A new direction in experiments is the creation of ultracompact frequency combs by way of nonlinear parametric optics in microresonators. We refer to these as microcombs, and here we report a silicon-chip-based microcomb optical clock that phase-coherently converts an optical-frequency reference to a microwave signal. A low-noise comb spectrum with 25 THz span is generated with a 2 mm diameter silica disk and broadening in nonlinear fiber. This spectrum is stabilized to rubidium frequency references separated by 3.5 THz by controlling two teeth 108 modes apart. The optical clocks output is the electronically countable 33 GHz microcomb line spacing, which features an absolute stability better than the rubidium transitions by the expected factor of 108. Our work demonstrates the comprehensive set of tools needed for interfacing microcombs to state-of-the-art optical clocks.

Self-Injection Locking and Phase-Locked States in Microresonator-Based Optical Frequency Combs

Microresonator-based optical frequency combs have been a topic of extensive research during the last few years. Several theoretical models for the comb generation have been proposed; however, they do not comprehensively address experimental results that show a variety of independent comb generation mechanisms. Here, we present frequency-domain experiments that illuminate the transition of microcombs into phase-locked states, which show characteristics of injection locking between ensembles of comb modes. In addition, we demonstrate the existence of equidistant optical frequency combs that are phase stable but with non-deterministic phase relationships between individual comb modes.

Laser-Machined Ultra-High-Q Microrod Resonators for Nonlinear Optics

Optical whispering-gallery microresonators are useful tools in microphotonics, and nonlinear optics at very low threshold powers. Here, we present details about the fabrication of ultra-high-Q whispering-gallery-mode resonators made by CO2-laser lathe machining of fused-quartz rods. The resonators can be fabricated in less than one minute and the obtained optical quality factors exceed Q = 10^9. Demonstrated resonator diameters are in the range between 170 {mu}m and 8 mm (free spectral ranges between 390 GHz and 8 GHz). Using these microresonators, a variety of optical nonlinearities are observed, including Raman scattering, Brillouin scattering and four-wave mixing.

Parametric seeding of a microresonator optical frequency comb

We have investigated parametric seeding of a microresonator frequency comb (microcomb) by way of a pump laser with two electro-optic-modulation sidebands. We show that the pump-sideband spacing is precisely replicated throughout the microcombs optical spectrum, and we demonstrate a record absolute line-spacing stability for microcombs of $1.6times10^{-13}$ at 1 s. The spectrum of a parametric comb is complex, and often non-equidistant subcombs are observed. Our results demonstrate that parametric seeding can not only control the subcombs, but can lead to the generation of a strictly equidistant microcomb spectrum.

Hybrid Electro-Optically Modulated Microcombs

Optical frequency combs based on mode-locked lasers have proven to be invaluable tools for a wide range of applications in precision spectroscopy and metrology. A novel principle of optical frequency comb generation in whispering-gallery mode microresonators (microcombs) has been developed recently, which represents a promising route towards chip-level integration and out-of-the-lab use of these devices. Presently, two families of microcombs have been demonstrated: combs with electronically detectable mode spacing that can be directly stabilized, and broadband combs with up to octave-spanning spectra but mode spacings beyond electronic detection limits. However, it has not yet been possible to achieve these two key requirements simultaneously, as will be critical for most microcomb applications. Here we present a key step to overcome this problem by interleaving an electro-optic comb with the spectrum from a parametric microcomb. This allows, for the first time, direct control and stabilization of a microcomb spectrum with large mode spacing (>140 GHz) with no need for an additional mode-locked laser frequency comb. The attained residual 1-second-instability of the microcomb comb spacing is 10^-15, with a microwave reference limited absolute instability of 10^-12 at a 140 GHz mode spacing.

Mechanical control of a microrod-resonator optical frequency comb

Robust control and stabilization of optical frequency combs enables an extraordinary range of scientific and technological applications, including frequency metrology at extreme levels of precision, novel spectroscopy of quantum gases and of molecules from visible wavelengths to the far infrared, searches for exoplanets, and photonic waveform synthesis. Here we report on the stabilization of a microresonator-based optical comb (microcomb) by way of mechanical actuation. This represents an important step in the development of microcomb technology, which offers a pathway toward fully-integrated comb systems. Residual fluctuations of our 32.6 GHz microcomb line spacing reach a record stability level of $5times10^{-15}$ for 1 s averaging, thereby highlighting the potential of microcombs to support modern optical frequency standards. Furthermore, measurements of the line spacing with respect to an independent frequency reference reveal the effective stabilization of different spectral slices of the comb with a $<$0.5 mHz variation among 140 comb lines spanning 4.5 THz. These experiments were performed with newly-developed microrod resonators, which were fabricated using a CO$_2$-laser-machining technique.